全文获取类型
收费全文 | 377篇 |
免费 | 5篇 |
国内免费 | 12篇 |
专业分类
安全科学 | 23篇 |
废物处理 | 17篇 |
环保管理 | 27篇 |
综合类 | 72篇 |
基础理论 | 86篇 |
污染及防治 | 115篇 |
评价与监测 | 32篇 |
社会与环境 | 19篇 |
灾害及防治 | 3篇 |
出版年
2023年 | 2篇 |
2022年 | 9篇 |
2021年 | 5篇 |
2020年 | 3篇 |
2019年 | 4篇 |
2018年 | 8篇 |
2017年 | 11篇 |
2016年 | 9篇 |
2015年 | 16篇 |
2014年 | 20篇 |
2013年 | 22篇 |
2012年 | 19篇 |
2011年 | 27篇 |
2010年 | 17篇 |
2009年 | 21篇 |
2008年 | 20篇 |
2007年 | 21篇 |
2006年 | 29篇 |
2005年 | 22篇 |
2004年 | 9篇 |
2003年 | 21篇 |
2002年 | 11篇 |
2001年 | 4篇 |
2000年 | 4篇 |
1999年 | 5篇 |
1998年 | 3篇 |
1997年 | 5篇 |
1995年 | 4篇 |
1994年 | 5篇 |
1990年 | 2篇 |
1987年 | 1篇 |
1986年 | 3篇 |
1985年 | 2篇 |
1984年 | 3篇 |
1982年 | 2篇 |
1981年 | 3篇 |
1980年 | 2篇 |
1977年 | 1篇 |
1975年 | 1篇 |
1971年 | 2篇 |
1970年 | 2篇 |
1969年 | 1篇 |
1966年 | 1篇 |
1963年 | 1篇 |
1962年 | 1篇 |
1956年 | 1篇 |
1954年 | 1篇 |
1950年 | 1篇 |
1941年 | 1篇 |
1936年 | 1篇 |
排序方式: 共有394条查询结果,搜索用时 31 毫秒
91.
Anne-Catherine Bénard Vincent Darcos Christian Drakides Claude Casellas Jean Coudane Michel Vert 《Journal of Polymers and the Environment》2011,19(1):40-48
Water-soluble synthetic polymers are extensively used in cosmetics, detergents and paints. Many end up in wastewater and,
later on, in wastewater-treatment plants. In order to gain an insight into their fate in such plants, fluorescence and radioactivity
labelings were compared using a lab-scale reactor designed to mimic industrial conditions. Two fermentation media were considered,
namely a mixture of E402 and E204 micro-organisms and an activated sludge collected from a water-treatment plant located in
the south of France. A sample of low molar mass commercial poly(acrylic acid) (PAA) was labeled by radioactivity with tritium
and by coupling the 6-aminofluorescein fluorescent dye. Labeled PAA-containing sludges were allowed to ferment. To monitor
the fate of the polymers, aliquots of the fermented mixtures were withdrawn at selected times and centrifuged. Liquid and
solid phases were analyzed by scintigraphy or UV spectrometry, depending of the labeling techniques. Both techniques led to
similar distributions, c.a. 75% in the supernatant and 25% in the solid phase. Distributions remained constant during the
biological tests. There was no degradation of the commercial PAA after aqueous size exclusion chromatography (SEC), in agreement
with literature. These features showed that fluorescence-labeling can be used instead of the complex and expensive radiolabeling.
The validated fluorescence-based method was then applied to a linear poly(acrylic acid) synthesized by ATRP and labeled with
6-aminofluorescein. There was no significant difference between the commercial and the linear poly(acrylic acid)s. In contrast,
a linear PAA with 5% of tert-butyl ester repeating units was predominantly found in the solid phase although adsorption or absorption by micro-organisms
could not be demonstrated. The method based on fluorescence labeling should be applicable to other water soluble polymers
provided that the dye remains attached to the polymer as it was the case for the studied poly(acrylic acid)s. 相似文献
92.
Directeur Gé né ral 《生态毒理学报》2001,23(1):38-42
布宜诺斯艾利斯市的增长伴随着环境的逐渐恶化,其中包括水流的质量 .随着情况的全面恶化, 1993年政府将饮用水厂进行了为期 30年的私有化,并在布宜诺斯艾利斯市及其 17个郊区社区进行净化处理 .阿瓜斯阿根廷斯 (Aguas Agentinas)的用水操作者是里昂水业集团,为了响应当局的要求,提出并着手进行净化处理的新指导模式,这有助于解决该承包区目前的环境问题 . 相似文献
93.
Jonathan D. Byer Michel Lebeuf Mehran Alaee Brown R. Stephen Steve Trottier Sean Backus Michael Keir Catherine M. Couillard John Casselman Peter V. Hodson 《Chemosphere》2013,90(5):1719-1728
The bioaccumulation of lipophilic contaminants such as polychlorinated biphenyls (PCBs), organochlorine pesticides (OCPs), and polybrominated diphenyl ethers (PBDEs) can result in a reduction in fitness and spawner quality in eels and may be a factor in Anguillid sp. population declines. Contaminant concentrations in eels have been studied extensively in Europe, but data for American eels are severely lacking. Concentrations of PCBs, OCPs, and PBDEs were determined in American eel from eastern Canada and New York, USA, along with European eel from Belgium. Principal component analysis revealed that eels captured in the St. Lawrence estuary were a mixture of upstream migrants from the St. Lawrence River watershed, and fish captured in local tributaries. Contaminant concentrations were dependent on origin, related to the local environment, and were lower than historic values. In Canada, concentrations of OCPs and PCBs in eel tissues were below the Canadian human consumption guidelines for contaminants in fish, indicating that the current risk to consumers is low. However, concentrations of PCBs, total DDT, and mirex in eels from L. Ontario and the upper St. Lawrence R. were above Great Lakes guidelines for the protection of piscivorous predators. Concentrations of penta-BDE homologs exceeded the Canadian guideline for environmental quality in over half of the eels in this study, but concentrations of the other homolog groups were below the guideline. 相似文献
94.
Michel C. Boufadel 《Journal of the American Water Resources Association》2000,36(1):203-213
ABSTRACT: Twenty storm events were used to select design values of the HEC1 loss parameters STRTL and CNSTL in order to route the probable maximum flood, PMF, through the Englewood watershed, Ohio. The parameter STRTL represents the initial volume of water lost due to interception and incomplete saturation of the soil prior to the storm. The parameter CNSTL represents a continuous loss rate and depends only on the watershed. When optimized from each storm event, STRTL varied between 0.0 and 3.4 inches with an average of 1.0 inch; CNSTL varied between 0.02 and 0.26 inch/hour, and it followed a normal probability distribution with a mean of about 0.1 inch/hour. The absence of correlation between optimum CNSTL values and each of total rainfall, total loss, and runoff duration supported the selection of the mean CNSTL as a design value. PMF routing through the Englewood watershed revealed that the PMF at the outlet is not sensitive to STRTL, but highly affected by CNSTL variations. The insensitivity to STRTL was due to the presence of a dam at the outlet of the watershed that caused the buildup of water in the watershed, thereby masking the storage effect of STRTL. The peak PMF increased by about 27 percent when the design CNSTL was decreased to 0.05 inch! hour, and decreased by about 18 percent when the design CNSTL was increased to 0.15 inch/hour. 相似文献
95.
96.
Maurike de Groot-van der Mooren Gert de Graaf Michel E Weijerman Mariette J. V Hoffer Jeroen Knijnenburg Anne-Marie M. F van der Kevie-Kersemaekers Angelique J. A Kooper Els Voorhoeve Birgit Sikkema-Raddatz Laura J. C. M van Zutven Malgorzata Ilona Srebniak Karin Huijsdens-van Amsterdam John J. M Engelen Dominique Smeets Anton H van Kaam Martina C Cornel 《黑龙江环境通报》2021,41(10):1351-1359
97.
Flipo N Jeannée N Poulin M Even S Ledoux E 《Environmental pollution (Barking, Essex : 1987)》2007,146(1):241-256
The objective of this work is to combine several approaches to better understand nitrate fate in the Grand Morin aquifers (2700 km(2)), part of the Seine basin. cawaqs results from the coupling of the hydrogeological model newsam with the hydrodynamic and biogeochemical model of river ProSe. cawaqs is coupled with the agronomic model Stics in order to simulate nitrate migration in basins. First, kriging provides a satisfactory representation of aquifer nitrate contamination from local observations, to set initial conditions for the physically based model. Then associated confidence intervals, derived from data using geostatistics, are used to validate cawaqs results. Results and evaluation obtained from the combination of these approaches are given (period 1977-1988). Then cawaqs is used to simulate nitrate fate for a 20-year period (1977-1996). The mean nitrate concentrations increase in aquifers is 0.09 mgN L(-1)yr(-1), resulting from an average infiltration flux of 3500 kgN.km(-2)yr(-1). 相似文献
98.
Nicole L. Michel Sarah P. Saunders Timothy D. Meehan Chad B. Wilsey 《Conservation biology》2021,35(5):1484-1495
Evaluation of protected area effectiveness is critical for conservation of biodiversity. Protected areas that prioritize biodiversity conservation are, optimally, located and managed in ways that support relatively large and stable or increasing wildlife populations. Yet evaluating conservation efficacy remains a challenging endeavor. We used an extensive community science data set, eBird, to evaluate the efficacy of protected areas for birds across the Gulf of Mexico and Atlantic coasts of the United States. We modeled trends (2007–2018) for 12 vulnerable waterbirds that use coastal areas during breeding or wintering. We compared two types of protected areas—sites where conservation organizations implemented active stewardship or management or both to reduce human disturbance (hereafter stewardship sites) and local, state, federal, and private protected areas managed to maintain natural land cover (hereafter protected areas)—as well as unprotected areas. We evaluated differences in trends between stewardship, protected, and unprotected areas across the Gulf and Atlantic coasts as a whole. Similar to a background sample, stewardship was known to occur at stewardship sites, but unknown at protected and unprotected areas. Four of 12 target species—Black Skimmer (Rynchops niger), Brown Pelican (Pelecanus occidentalis), Least Tern (Sternula antillarum), and Piping Plover (Charadrius melodus)—had more positive trends (two to 34 times greater) at stewardship sites than protected areas. Furthermore, five target species showed more positive trends at sites with stewardship programs than unprotected sites during at least one season, whereas seven species showed more positive trends at protected than unprotected areas. No species had more negative trends at stewardship sites than unprotected areas, and two species had more negative trends at protected than unprotected areas. Anthropogenic disturbance is a serious threat to coastal birds, and our findings demonstrate that stewardship to reduce its negative impacts helps ensure conservation of vulnerable waterbirds. 相似文献
99.
Florence Censier Christophe Y. Fischer Sandrine Chavalle Stephanie Heuskin Marie-Laure Fauconnier Bernard Bodson Michel De Proft Georges C. Lognay Pascal Laurent 《Chemoecology》2014,24(6):243-251
The saddle gall midge, Haplodiplosis marginata (von Roser) (Diptera: Cecidomyiidae), has undergone a resurgence recently as a pest of cereals in Belgium and other European countries. An effective monitoring tool of saddle gall midge flights is needed to understand the enigmatic population dynamics of this pest, and to design an integrated management strategy. Therefore, volatile compounds emitted by females (alkan-2-ols and alk-2-yl butanoates) were identified, and the chirality of the emitted esters was determined to be the R absolute configuration. In field-trapping experiments, racemic non-2-yl butanoate attracted substantial numbers of H. marginata males. Thus, this compound will be useful in baited traps for monitoring seasonal flight patterns, and improving integrated management of the saddle gall midge in agricultural systems. 相似文献
100.
Sophie Gauthier-Clerc Isabelle Boily Michel Fournier Karine Lemarchand 《Environmental science and pollution research international》2013,20(2):612-620
Mussels are widespread in coastal environments and experience various physical, chemical, and bacteriological conditions. Owing to the increase of coastal urbanization, mussels are now commonly exposed not only to indigenous bacteria, but also to enteric bacteria originating from pulsed and chronic sewage discharges into coastal environments. Due to its broad resilience to environmental variations, the blue mussel Mytilus edulis is commonly used as an indicator of environmental quality in bio-monitoring programs. However, since mussel immune system capabilities may be affected by the presence of exogenous fecal bacteria in coastal seawater subjected to sewage discharges, we aimed to determine the effect of in vivo bacterial challenges on mussels' immune competency by using two exogenous enteric bacterial strains, Escherichia coli and Enterococcus faecalis, and an indigenous bacterial strain Vibrio splendidus (as control). Bacterial strains were tested individually, by injection into the posterior adductor muscle at three different cell densities (102, 103, and 104 cells). Unlike classic in vitro experiments using higher bacterial concentrations, neither the enteric bacteria nor the indigenous strain induced significant increase or decrease of either cell-mediated (phagocytosis, reactive oxygen species, and NO x production) or humoral components (prophenoloxidase-like, acid phosphatase, and l-leucine-aminopeptidase production) of the immune system. This study demonstrates that, at low concentrations, E. coli and E. faecalis do not represent an additional threat that could impair M. edulis immune competency and, as a consequence, its potential of survival in coastal areas subjected to sewage discharges. 相似文献